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Rotational Spectrum of the AsH₂ Radical in Its Ground State, Studied by Far-Infrared Laser Magnetic Resonance

Author： Hughes R.A. Brown J.M. Evenson K.M.

Publisher： Academic Press

ISSN： 0022-2852

Source： Journal of Molecular Spectroscopy, Vol.200, Iss.2, 2000-04, pp. : 210-228

Disclaimer: Any content in publications that violate the sovereignty, the constitution or regulations of the PRC is not accepted or approved by CNPIEC.

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Abstract

The rotational spectrum of AsH₂ in its ground X~²B₁ electronic state has been recorded using a far-infrared laser magnetic resonance spectrometer. The AsH₂ radical was produced inside the spectrometer cavity by the reaction of arsine (AsH₃) with fluorine atoms. Hyperfine splittings from both ⁷⁵As and ¹H nuclei were observed, and analysis of the spectra has yielded accurate values for rotational, hyperfine, and Zeeman parameters.

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