Core‐Structure‐Motivated Design of Iminium–Enolate Organocascade Reactions: Enantioselective Syntheses of 5,6‐Dihydroindolizines

Publisher： John Wiley & Sons Inc

E-ISSN： 1521-3757|125|35|9431-9435

ISSN： 0044-8249

Source： ANGEWANDTE CHEMIE, Vol.125, Iss.35, 2013-08, pp. : 9431-9435

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Abstract

Indolizin‐Gerüste: Ein hocheffizienter doppelter Bildungs‐ und Aktivierungsprozess von Iminiumenolaten wird vorgestellt und zur Entwicklung organokatalytischer intermolekularer Dominoreaktionen für die direkte Synthese von 5,6‐Dihydroindolizinen verwendet. Dieser von einfachen Edukten ausgehend Prozess bietet einfachen Zugang zu Indolizin‐Gerüsten mit hoher optischer Reinheit (siehe Bild).

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