

Publisher: Edp Sciences
E-ISSN: 2100-014x|41|issue|12005-12005
ISSN: 2100-014x
Source: EPJ Web of Conference, Vol.41, Iss.issue, 2013-03, pp. : 12005-12005
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Abstract
The third harmonic of a few-cycle pulse, generated at different dielectric surfaces, is investigated using interferometric frequency-resolved optical gating. We present direct experimental evidence for a non-instantaneous nonlinear response in a TiO2 thin film whereas surface third-harmonic generation in a SiO2 sample does not show any indication for non-instanteneity. To the best of our knowledge, this constitutes the first report of a non-instantaneous nonlinear optical response of a dielectric optical material.
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