Exciton-exciton scattering in a one-dimensional J aggregate

Author: Abramavicius D.  

Publisher: Edp Sciences

E-ISSN: 1286-4854|101|5|57007-57007

ISSN: 0295-5075

Source: EPL (EUROPHYSICS LETTERS), Vol.101, Iss.5, 2013-03, pp. : 57007-57007

Disclaimer: Any content in publications that violate the sovereignty, the constitution or regulations of the PRC is not accepted or approved by CNPIEC.

Previous Menu Next

Abstract

The exciton scattering approach is applied to describe an exciton-exciton interaction problem in an excitonic linear aggregate. An analytic expression for the scattering amplitude is derived for an infinite periodic system. The result allows to obtain a typical spectral lineshape of the main resonance of the J aggregate in the coherent third-order two-dimensional spectra. The obtained functional form of the scattering allows to suggest a universal expression of the scattering amplitude for delocalized excitons in realistic systems.