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Thermochemical Insights into Fullerene Aggregation and the Phthalocyanine–Fullerene Interaction in Efficient Solvents

Publisher： John Wiley & Sons Inc

E-ISSN： 1439-7641|19|3|284-290

ISSN： 1439-4235

Source： CHEMPHYSCHEM, Vol.19, Iss.3, 2018-02, pp. : 284-290

Disclaimer: Any content in publications that violate the sovereignty, the constitution or regulations of the PRC is not accepted or approved by CNPIEC.

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Abstract

AbstractThe physicochemical behavior of fullerene C₆₀ in hydrocarbon solvents is examined by isothermal titration calorimetry, photocalorimetry, and UV spectroscopy. The obtained data are summarized to substantiate the idea of the binary fullerene/solvent cluster as a colloidal nanoentity that moderates noncovalent interactions of the C₆₀ molecule in solution. This idea serves to aid understanding of the complex physicochemical behavior of tert‐butyl‐substituted phthalocyanine in C₆₀‐saturated o‐xylene under illumination with low‐energy photons. The proposed experimental approach, which focuses on concentrated solutions and is applicable to multicomponent systems, is discussed as a potential tool of materials science.

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