Optical Spectroscopy of Perovskite-Type Manganites

Author: Okimoto Y.  

Publisher: Springer Publishing Company

ISSN: 0896-1107

Source: Journal of Superconductivity: Incorporating Novel Magnetism, Vol.13, Iss.2, 2000-04, pp. : 271-284

Disclaimer: Any content in publications that violate the sovereignty, the constitution or regulations of the PRC is not accepted or approved by CNPIEC.

Previous Menu Next

Abstract

Review is given on late optical studies on colossal magnetoresistance (CMR) manganites with perovskite or related structures. In La_1−xSr_xMnO_3 which undergoes a ferromagnetic transition, optical conductivity spectrum () shows a change from a gap-like feature to metallic but highly diffussive one with increasing spin-polarization. Such a remarkable spectral weight transfer is also observed in a layered manganite, La_2−2xSr_1+2xMn_2O_7 (x = 0.4), with a mid-infrared peak structure due to inter-orbital (d_{x^2-y^2} → d_{3z^2-r^2}) transition. In Pr_1−xCa_xMnO_3 (x = 0.4) which undergoes the charge ordering phase transition, () shows an anisotropic feature reflecting charge/orbital ordering pattern at 10 K. The charge-ordered state is transformed into a ferromagnetic metallic state by a magnetic field of 6.5 T at 30 K, which is manifested in a huge change of optical spectra over a wide photon-energy region (0.05 eV–3 eV).