Palladium/Copper‐Catalyzed Oxidative CH Alkenylation/N‐Dealkylative Carbonylation of Tertiary Anilines

Publisher： John Wiley & Sons Inc

ISSN： 0044-8249

Source： ANGEWANDTE CHEMIE, Vol.125, Iss.40, 2013-09, pp. : 10776-10779

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Abstract

C‐H/C‐N‐Aktivierung: Die erste Palladium/Kupfer‐katalysierte aerobe oxidative C‐H‐Alkenylierung/N‐desalkylierende Carbonylierung von tertiären Anilinen wurde entwickelt. Die Reaktion ist mit vielen funktionellen Gruppen kompatibel, kann auch Acrylester umsetzen und ermöglichte die effiziente Synthese von biologisch aktiven 3‐Methylenindolin‐2‐onen aus preiswerten und einfachen Substraten.

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